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CLBO

當前位置： 首頁 ? Products ? 非線性晶體 ? CLBO
CLBO

CLBO(硼酸銫鋰，CsLiB6O10)是一種新型的非線性晶體。它的透明光譜范圍寬（175~2800nm），非線性系數高，是KDP的2.2倍，離散角小。激光破壞閥值高，達26GW/cm2，倍頻轉換效率達60%（SHG）。

可以在室溫工作，很適合Nd:YAG激光器產生4w（266nm）和5w（213nm）倍頻光輸出?？捎糜谧贤鈪⒘空袷帲∣PG）和參量放大（OPA）。

特點

  • 小離散角；
  • 低吸收系數；
  • 高頻轉換效率；
  • 容易長大的單晶；
  • 高激光損傷閾值；
  • 高效非線性光學系數；
  • 其紫外線吸收邊緣達到180 nm；
  • 較大的角度，光譜和溫度帶寬值；

物理和化學特性

屬性數值
化學式CsLiB6O10
晶體結構四方負單軸晶體，42 m
晶格常數a=10.494?,c = 8.939?,Z=4
質量密度2.461 g/cm3
莫氏硬度5.5
熔點1118 K
分子質量364.706
導熱系數1.25 W/m K

非線性光學性質

屬性數值
NLO系數deff(I)=d36sinθmsin(2φ)
?deff(II)=d36sin(2θm)cos(2φ)
熱光系數dno/dT=-1.9*10-6/℃
?dne/dT=-0.5*10-6/℃
損傷閾值26 GW/cm2
波長（nm）532 + 532 = 266
1064 + 266 = 213
相位匹配角（°）61.7
68.4
流量（pm / V）0.84
0.87
角度公差（mrad·cm）0.49
0.42
偏角（°）1.83
1.69
光譜接受度（nm·cm）0.13
0.16
溫度接受度（℃·cm）8.3
4.6

線性光學性質

屬性Value
透明范圍180-2750 nm
吸收系數0.0013 cm?1
折光指數
1.064微米ne?= 1.4340, no?= 1.4838
0.532微米ne?= 1.4445, no?= 1.4971
??
Sellmeier方程（λinμmno2?= 2.2104+0.01018/(λ2-0.01424)-0.01258λ2
ne2?= 2.0588+0.00838/(λ2-0.01363)-0.00607λ2

折光指數的實驗值

λ[μm]none
0.421.50581.4517
0.451.5031.4493
0.481.50061.4474
0.51.49911.4462
0.5321.49711.4445
0.561.49571.4434
0.591.49431.4422
0.611.49351.4414
0.63281.49281.4409
0.671.49151.4398
0.71.49071.4392
0.721.49021.4387
1.0641.48381.434

相位匹配溫度，內部角度和溫度帶寬的實驗值

相互作用波長[μm]θpm [deg]T [?C]Δθint?[deg]ΔT [?C]
SHG, o + o???e
0.946???0.47390-15?5
0.5235???0.2617565.8~160??
0.5321???0.2660562~140??
61.4200.236.2
1.0642???0.532129.5200.04352.7
1.3382???0.669127.720?68.7
SFG, o + o???e
1.0642 + 0.26605???0.2128467.320?3.6
1.547 + 0.221???0.1933861.7150??
1.9079 + 0.2128???0.19145520?1.2
1.0642 + 0.35473???0.2660550.620?6.1
1.0642 + 0.5321???0.3547339.120?18
SHG, e + o???e
1.0642???0.532142.420?49.4
SFG, e + o???e
1.9079 + 0.2128???0.191457.420?1.1
1.0642 + 0.5321???0.3547348.920?17

光譜

二次諧波轉換效率與輸入基本脈沖能量的函數的計算結果

CLBO透射光譜

折射率色散

I和II型的相位匹配角隨基波波長的變化

參考文獻

[1]? Kawamura T ,? Yoshimura M ,? Shimizu Y , et al. Crystal growth of CsLiB6O10CsLiB6O10 in a dry atmosphere and from a stoichiometric melt composition[J]. Journal of Crystal Growth, 2010, 312(8):1118-1121.
[2] AE Kokh,? Kononova N G ,? Lisova I A , et al. CsLiB6O10 crystal: forth and fifth-harmonic generation in Nd:YAP laser[J]. Proceedings of SPIE – The International Society for Optical Engineering, 2001, 4268.
[3]? Lv X ,? Yuan J L ,? Dai Y , et al. Study on Ultra-Precise Machining of CLBO Crystal[J]. Key Engineering Materials, 2006, 304-305:398-402.
[4]? Mori Y ,? Kuroda I ,? Nakajima S , et al. New nonlinear optical crystal: Cesium lithium borate[J]. Applied Physics Letters, 1995, 67(13):1818-1820.
[5]? Ryu G ,? Yoon C S ,? Han T , et al. Growth and characterisation of CsLiB6O10 (CLBO) crystals[J]. Journal of Crystal Growth, 1998, 191(3):492-500.
[6]? Sasaki T ,? Mori Y ,? Kuroda I , et al. Caesium Lithium Borate: a New Nonlinear Optical Crystal[J]. Acta Crystallographica, 2010, 51(11):2222-2224.
[7]? Sekine T ,? Sakai H ,? Takeuchi Y , et al. High efficiency 12.5 J second-harmonic generation from CsLiB6O10 nonlinear crystal by diode-pumped Nd:glass laser[J]. Optics Express, 2013, 21(7):8393-8400.
[8]? Yu X ,? Hu Z G . Flux growth of CsLiB6O10 crystals[J]. Journal of Crystal Growth, 2010, 312(16-17):2415-2418.
[9]? Yuan X ,? Shen G ,? Wang X , et al. Growth and characterization of large CLBO crystals[J]. Journal of Crystal Growth, 2006, 293(1):97-101.
[10]? Bhar G C ,? Kumbhakar P ,? Chatterjee U , et al. Widely tunable deep ultraviolet generation in CLBO[J]. Optics Communications, 2000, 176(1-3):199-205.
[11]? Ono R ,? Kamimura T ,? Fukumoto S . Effect of crystallinity on the bulk laser damage and UV absorption of CLBO crystals[J]. Journal of Crystal Growth, 2002, 237:645-648.
[12]? Mori Y ,? Kuroda I ,? Nakajima S , et al. Growth of a nonlinear optical crystal: cesium lithium borate[J]. Journal of Crystal Growth, 1995, 156(3):307-309.
[13]? Mirov S B ,? Fedorov V V ,? Boczar B , et al. All-solid-state laser system tunable in deep ultraviolet based on sum-frequency generation in CLBO[J]. Optics Communications, 2001, 198(4-6):403-406.
[14]? Pylneva N A ,? Kononova N G ,? Yurkin A M , et al. Top-seeded solution growth of CLBO crystals[J]. Proceedings of SPIE – The International Society for Optical Engineering, 1999, 3610:148-155.
[15]? Yap Y K ,? Inagaki M ,? Nakajima S , et al. High-power fourth- and fifth-harmonic generation of a Nd:YAG laser by means of a CsLiB(6)O(10).[J]. Optics Letters, 1996, 21(17):1348.
[16]? Sakuma J ,? Asakawa Y ,? Obara M . Generation of 5-W deep-UV continuous-wave radiation at 266 nm by an external cavity with a CsLiB6O10 crystal[J]. Optics Letters, 2004, 29(1):92-4.
[17] Trnovcova, V, Fedorov, et al. Electrical and dielectric properties of b-BaB2O4 (BBO) and CsLiB6O10 (CLBO) crystals[J]. Journal of Physics & Chemistry of Solids, 2007.
[18]? Yap Y K ,? Inoue T ,? Sakai H , et al. Long-term operation of CsLiB6O10 at elevated crystal temperature[J]. Optics Letters, 1998, 23(1):34.
[19]? Yap Y K ,? Haramura S ,? Taguchi A , et al. CsLiB6O10 crystal for frequency doubling the Nd:YAG laser – ScienceDirect[J]. Optics Communications, 1998, 145( 1–6):101-104.
[20]? Bowers M S ,? Trautmann T M ,? Gerstenberger D C . Non-critically phase-matched second-harmonic generation in cesium lithium borate[C]// Advanced Solid-State Photonics. Aculight Corporation, 11805 North Creek Parkway South # 113 Bothell, Washington 98011, 2003.
[21]? Mori Y ,? Yap Y K ,? Kamimura T , et al. Recent development of nonlinear optical borate crystals for UV generation[J]. Optical Materials, 2002, 19(1):1-5.
[22]? Bai K ,? Jung S T . Growth and characterization of pure and Er-doped CsLiB 6O 10 single crystals[J]. Journal of Crystal Growth, 1998, 186(4):612-615.
[23]? Chandra S ,? Allik T H ,? Hutchinson J A , et al. Tunable ultraviolet laser source based on solid-state dye laser technology and CsLiB6O10 harmonic generation[J]. Optics Letters, 1997, 22(4).
[24]? Zhou W L ,? Mori Y ,? Sasaki T , et al. High-efficiency intracavity continuous-wave ultraviolet generation using crystals CsLiB~6O~1~0, -BaB~2O~4 and LiB~3O~5[J]. OPTICS COMMUNICATIONS, 1996, 123(4).
[25]? Yushi K ,? Yarborough J M ,? Li L , et al. Continuous-wave all-solid-state 244 nm deep-ultraviolet laser source by fourth-harmonic generation of an optically pumped semiconductor laser using CsLiB6O10 in an external resonator[J]. Optics Letters, 2008, 33(15):1705-7.
[26]? Petrov V ,? Noack F ,? Rotermund F . Sum-Frequency Generation of Femtosecond Pulses in CsLiB(6)O(10) Down to 175 nm.[C]// Conference on Lasers & Electro-optics. 2000.
[27]? Sakuma J ,? Finch A ,? Ohsako Y , et al. High-power narrowband DUV laser source by frequency mixing in CLBO[J]. International Society for Optics and Photonics, 2000, 3889:516-523.
[28]? Nishioka M ,? Kanoh A ,? Yoshimura M , et al. Growth of CsLiB 6O 10 crystals with high laser-damage tolerance[J]. J.cryst.growth, 2005, 279(1-2):76-81.

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